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  • Primary Radiation Damage Cross Sections

    Closed for proposals

    Project Type

    Coordinated Research Project

    Project Code

    F44003

    CRP

    1968

    Approved Date

    13 December 2012

    Status

    Closed

    Start Date

    3 May 2013

    Expected End Date

    2 May 2018

    Completed Date

    12 July 2018

    Description

    The radiation damage in the materials is? a key parameter that eventually defines the life expectancy and safety operation of?the nuclear facilities. The time evolution and final appearance of material changes depend?on the type, intensity?and energy spectra of incident radiation?as well as?on the materials properties and ambient environment. Although this?process is not yet?completely understood, it has been established?that some material property changes are sensitive to the results of nuclear collisions (atom displacement and?gas production), while others are more sensitive to the effects of ionization. ?For the group of practically important materials with crystalline structure, such as metals, ceramics?and some alloys, the atom displacement cross section was found to be a reference?parameter?suitable for?characterization and comparison of the radiation damage induced by neutrons and charged particles. ?The so-called NRT-dpa standardproposed by Norget, Torrens and Robinson for evaluation of the number of displaced atoms? has been universally used since 1975. Although the usefulness of the NRT-dpa for correlating many radiation damage phenomena was recognized, its limitations were also demonstrated with?indications that other parameters?could be used to better correlate certain kinds of data. ?The development of specific damage models is best done within the materials community, based on information obtained from nuclear data researchers. For a given irradiation environment, these data need to include the primary knock-on atom (PKA) spectrum, nuclear transmutation rates (particularly gas production), and partitioning of the PKA energy into nuclear and electronic stopping effects.?This CRP engages participants from both the nuclear data and materials research communities and will?determine the best possible parameter (or a few parameters) for correlating damage from irradiation facilities with very different particle types and energy spectra, including fission and fusion reactors, charged particle accelerators, and spallation irradiation facilities. The essential progress?in the course of?CRP?is expected for crystalline materials (such as fuel UO2, structural metals, SiC), for which?the upgraded cross sections for the?primary damage (primary radiation defects and gas production)?will be produced.

    Objectives

    To find ways to?overcome the drawbacks, limitations?of the NRT-dpa relying on recent/modern developments in primary radiation damage simulations. For this, engage in this project experts from the nuclear data and material research communities together to:revisit the NRT-dpa protocols, improve recoil and emitted particles spectra?treatments, account for?uncertainties, propose new metrics, extend the energy range;elaborate upgraded primary radiation defect?metrics to better capture the annealing, evolution?of defects in the recoil cascades on the basis of MD, BCA and other models;demonstrate?better metrics?to correlate?experimental (ions based)?to model?parameters (neutron based) for microstructural material damage;review, enhance?gas production from evaluated nuclear data?files?and make recommendations.

    Specific objectives

    - Encourages, entices?the nuclear data/processing?and materials research communities to?more efficiently?work together, develop?better metrics and models. - Engage the true multi-scale (atom/isotope-molecule/element-alloy/material) aspects of characterising?materials?properties evolution?under particles?irradiation. - Provide, elaborate and engineer more robust methodologies able to cover all experimental and modelling?aspects of study of materials under ions and neutron irradiations.?Most experimental information are based on ions, while the next generation devices will endure high energy neutrons.?- Develop the physics and metrics to bridge the gaps.

    Impact

    This Coordinated Research Project was aimed at reviewing the theory, methodology and data-streams behind the ubiquitous NRT-dpa material damage-dose-defect cross-section–based metric, including its short-comings. Furthermore, the project aimed to evaluate and explore alternative, modern and enhanced metrics that (theoretically) could be better able to highlight the complex problem of correlating, simulating and predicting the behavior an evolution of materials properties when under particle irradiation. It reached and on occasion surpassed all expectations

    Relevance

    The development and usage of traditional and novel nuclear materials with improved properties and functionalities are key requirements to provide solutions to major modern engineering challenges in most nuclear applications

    CRP Publications

    Type

    Articles, reports

    Year

    2013 - 2019

    Publication URL

    https://www-nds.iaea.org/CRPdpa/CRP_Publications.pdf

    Country/Organization

    All participant, country

    Type

    Nuclear Materials and Energy 9 576–580, March 2016

    Year

    March 2016

    Publication URL

    http://fispact.ukaea.uk/wp-content/uploads/2017/01/gilbert_sublet_nucl_mater_ene…

    Description

    M.R. Gilbert, J.-Ch. Sublet. PKA distributions: Contributions from transmutation products and from radioactive decay.

    Country/Organization

    United Kingdom

    Type

    Eur. Phys. J. Plus (2019) 134: 350 DOI 10.1140/epjp/i2019-12758-y

    Year

    2019

    Publication URL

    https://epjplus.epj.org/articles/epjplus/abs/2019/07/13360_2019_Article_12758/13…

    Description

    Neutron-induced damage simulations: Beyond defect production cross-section, displacement per atom and iron-based metrics

    Country/Organization

    The European Physical Journal Pus

    Type

    Culham Centre for Fusion Energy

    Year

    2016

    Publication URL

    http://fispact.ukaea.uk/documentation-2/reports/

    Description

    Handbook of activation, transmutation and radiation damage properties of the elements simulated using FISPACT-II & TENDL-2015; Magnetic Fusion Plants CCFE-R(16)36

    Country/Organization

    United Kingdom

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